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Catalytic and Process Study of the Selective Hydrogenation of Acetylene and 1,3-Butadiene

Medium: Buch
ISBN: 978-981-10-9247-3
Verlag: Springer Nature Singapore
Erscheinungstermin: 07.07.2018
Lieferfrist: bis zu 10 Tage

This thesis offers novel methods for catalyst and process design for the selective hydrogenation of acetylene and 1,3-butadiene. The author predicts the properties of supported Pd–Ni bimetallic catalysts using density functional theory (DFT) calculations and temperature-programmed desorption (TPD). The excellent correlation between model surfaces and supported catalysts demonstrates the feasibility of designing effective bimetallic catalysts for selective hydrogenation reactions. The author also proposes a method for designing non-precious metal catalysts to replace precious metals. She modifies the process of selective hydrogenation of acetylene by coupling the selective adsorption to the selective hydrogenation in the liquid phase, as a result of which the ethylene selectivity is greatly improved and heat transfer is greatly enhanced. Lastly, by analyzing the mechanism of liquid-phase hydrogenation, the author proposes a multi-stage slurry bed reactor for industrial applications.<


Produkteigenschaften


  • Artikelnummer: 9789811092473
  • Medium: Buch
  • ISBN: 978-981-10-9247-3
  • Verlag: Springer Nature Singapore
  • Erscheinungstermin: 07.07.2018
  • Sprache(n): Englisch
  • Auflage: Softcover Nachdruck of the original 1. Auflage 2017
  • Serie: Springer Theses
  • Produktform: Kartoniert, Previously published in hardcover
  • Gewicht: 248 g
  • Seiten: 141
  • Format (B x H x T): 155 x 235 x 9 mm
  • Ausgabetyp: Kein, Unbekannt
Autoren/Hrsg.

Autoren

Introduction.- Experimental and Theoretical Methods.- Design of Pd-Ni Bimetallic Catalyst.- Effect of Oxide Supports on Pd–Ni Bimetallic Catalysts.- Replacing Precious Metals with Carbide Catalysts.- Liquid Phase Hydrogenation of Acetylene.- Conclusion.